I can't help with linking Charles Carroll with the VA Carrolls but I'm wondering if your Samuel is the brother to my ggggrand dad Daniel Boone Carroll. If so their parents were Luke Carroll and Martha Noland according to one family tree I found. I'm related to Daniel and Rebecca ???, Daniels second wife Mary Ann Sturgill was born in Russell county VA so I'm hoping we are of the same line and you have more on our ancestors.
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